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Synergistic effect of the sequential use of UV irradiation and chlorine to disinfect reclaimed water

机译:依次使用紫外线和氯气对再生水进行消毒的协同效应

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摘要

The effectiveness of UV and chlorination, used individually and sequentially, was investigated in killing pathogenic microorganisms and inhibiting the formation of disinfection by-products in two different municipal wastewaters for the source water of reclaimed water, which were from a microfilter (W1) and membrane bioreactor (W2) respectively. Heterotrophic plate count (HPC), total bacteria count (TBC), and total coliform (TC) were selected to evaluate the efficiency of different disinfection processes. UV inactivation of the three bacteria followed first-order kinetics in W1 wastewater, but in W2 wastewater, the UV dose response curve trailed beyond approximately 10 mJ/cm(2) UV. The higher number of particles in the W2 might have protected the bacteria against UV damage, as UV light alone was not effective in killing HPC in W2 wastewater with higher turbidity. However, chlorine was more effective in W2 than in W1 for the three bacteria inactivation owing to the greater formation of inorganic and organic chloramines in W1 wastewater. Complete inactivation of HPC in W1 wastewater required a chlorine dose higher than 5.5 mg/L, whereas 4.5 mg/L chlorine gave the equivalent result in W2 wastewater. In contrast, sequential UV and chlorine treatment produced a synergistic effect in both wastewater systems and was the most effective option for complete removal of all three bacteria. UV disinfection lowered the required chlorine dose in W1, but not in W2, because of the higher chlorine consumption in W2 wastewater. However, UV irradiation decreased total trihalomethane formation during chlorination in both wastewaters. (C) 2011 Elsevier Ltd. All rights reserved.
机译:分别研究了紫外线和氯化作用的有效性,分别用于依次消毒微生物和抑制两种不同市政废水中再生水的原水的消毒副产物的形成,这些废水来自微滤器(W1)和膜生物反应器(W2)。选择异养平板数(HPC),总细菌数(TBC)和总大肠菌群(TC)来评估不同消毒过程的效率。在W1废水中,这三种细菌的UV失活遵循一级动力学,但是在W2废水中,UV剂量响应曲线已超过约10 mJ / cm(2)UV。 W2中较高数量的颗粒可能已保护细菌免受紫外线伤害,因为仅紫外线对杀死浊度较高的W2废水中的HPC无效。然而,由于W1废水中更多的无机和有机氯胺形成,氯在W2中比W1在三种细菌灭活方面更有效。 W1废水中的HPC完全灭活需要氯剂量高于5.5 mg / L,而4.5 mg / L的氯在W2废水中具有相同的结果。相比之下,顺序的紫外线和氯气处理在两种废水系统中均产生协同效应,是完全去除所有三种细菌的最有效选择。紫外线消毒降低了W1中所需的氯剂量,但降低了W2中所需的氯剂量,因为W2废水中的氯消耗量更高。但是,紫外线照射减少了两种废水在氯化过程中总三卤甲烷的形成。 (C)2011 Elsevier Ltd.保留所有权利。

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